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Shirogane no Soleil was the first Soleil game and the one that defined the most essential elements of how the Runes, Valkyries, and other elements were treated within the multiverse (though a lot has been retconned since then). It is also a very old-style chuunige. The protagonist starts out as a normie, the girls are more powerful than him, and there is a horrible cost for using their powers. The heroines will seem somewhat archetypical in comparison to modern chuunige heroines, but that doesn't hurt the game as much as you would think. If you intend to play other games in the series, you should also pay attention to what happens to the various heroines, as some of it 'ripples' outward through the multiverse and has effects on their alternative versions.